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The steady state and time resolved spectroscopic properties of a series of donor-acceptor substituted phenylpyridines, where the phenylpyridines contain coordination sites that are redox-active, have been investigated. The steady state fluorescence of the donor excited states has been observed in the phenylpyridines with naphthalene (1a) and phenanthrene (1b), whereas no fluorescence was detected in the phenylpyridine with chrysene (1c). The time resolved fluorescence of the donor excited states has been observed in the phenylpyridines with 1a and 1b, indicating that fluorescence occurs through electron transfer from the redox-active metal centre. Time resolved fluorescence of 1a in acetonitrile and benzonitrile has been observed, demonstrating that energy transfer can occur between the ligand and the metal centre in these solvent systems. For 1a in methanol and pyridine, no direct excitation of the metal centre from either excited state of the donor has been observed, demonstrating that energy transfer from the donor excited state to the metal centre occurs through a vibrationally coupled intermediate, forming a twisted state.Coronavirus: Is it just a cold or is it the ‘big one’?
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DELPHI: Do you think coronavirus is just a flu or is it really the “Big one”?
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THE GATEWAY – MEMOIRS OF A VISIONARY TELECONNECTICUT by Thom Gunn; edited and with an introduction by Charles Simic. (Feb 2007, 141pp, $13.95). Growing up in the eighteenth century, Thom Gunn experienced a great deal. Born in 1890 in Jeddah, he lived in the city until age 7, when he entered Quaker school with his brother Edward, who would become a poet as well. During the years of the Edwardian twilight, the family moved back to England, where Thom and his brother spent their school years. The Europeanization of Britain seemed to intensify the classicism that was already their father’s inheritance.
While preparing for theological study at Emmanuel College, Cambridge, Thom spent a year in Switzerland. Here he first began to feel the true size of Nature, and to sense the inexhaustibility of the universe. “That year,” he later remembered, “I had the passion of an Outsider.” Following Cambridge, he continued reading and studying. He traveled to India, where he studied Sanskrit. On Christmas Day, 1911, while he was in Austria, he suddenly and involuntarily experienced an illumination, as if he had been dreaming and had wakened to find that he was awake and “at home” in the universe. He was twenty-six. The influence of this event and the people he met in India and in Vienna later penetrated his poetry in a most extraordinary way. During World War I he held a commission in the Royal Naval Air Service, serving at Dunkirk.
Initially he was a professional pilot; later he used his writings to express the poetry of air travel. After the war, he went on to study and work in Cambridge with Lawrence Sterne, whom he revered. Throughout his life, he pursued an extraordinary web of friendships, both professional and personal, through decades of travel, work, and residence in England, France, Italy, Austria, Switzerland, Germany, Germany, Arabia, and India. His poetry is expressed in many forms: books of verse, pamphlets, plays, literary criticism, essays, sketches, and several volumes of autobiographical prose and correspondence. Thom Gunn is regarded as one of the founders of the poetry of the first third of the twentieth century. In all his works, perhaps most clearly in The Uses of Poetry and Voices (1966), he contemplates the value and importance of poetry in a pervasive naturalism that can be applied to the arts of everything else. The majority of
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